Layered 2D (PbI2)1−
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Abstract x (BiI3)x materials exhibit a nonlinear dependence in structural and charge transport properties unanticipated from the combination of PbI2and BiI3. Within (PbI2)1−x (BiI3)x crystals, phase integration yields deceptive structural features, while phase boundary separation leads to new conductance switching behavior observed as large peaks in current during current–voltage (I –V ) measurements (±100 V). Temperature‐ and time‐dependent electrical measurements demonstrate that the behavior is attributed to ionic transport perpendicular to the layers. High‐resolution transmission electron microscopy reveals that the structure of (PbI2)1−x (BiI3)x is a “brick wall” consisting of two phases, Pb‐rich and Bi‐rich. These brick‐like features are 10s nm a side and it is posited that iodide ion transport at the interfaces of these regions is responsible for the conductance switching action. -
Trócoli, Rafael ; Parajuli, Prakash ; Frontera, Carlos ; Black, Ashley P. ; Alexander, Grant C. B. ; Roy, Indrani ; Arroyo-de Dompablo, M. Elena ; Klie, Robert F. ; Cabana, Jordi ; Palacín, M. Rosa ( , ACS Applied Energy Materials)